Introduction. Catalytic coal gasification has been studied worldwide for nearly 20 years due to its advantages, such accelerating process rate, improving carbon conversion degree, reducing process temperature, and thus decreasing energy consumption and limiting mechanical problems due to moderate conditions in a gasifier, as well as achieving a desired gas composition (Huang et al., 2015).
In this study, DFT is used to search for possible CO2 gasification paths at the two char edges (armchair edge and zigzag edge) catalyzed by Fe. The optimal reaction path is determined by path ...
Abstract. Catalytic gasification of a Wyodak lowsulfur subbituminous coal from the Powder River Basin of Wyoming was investigated using an inexpensive catalyst, Na2CO3, widely available in ...
The catalytic gasification of coal using calcium as the catalyst has several advantages over potassium, such as lower costs and corrosiveness, abundant reserves on earth, and facile accessibility. ... 2015 Reaction kinetics of Powder River Basin coal gasification in carbon dioxide using a modified drop tube reactor. Fuel 140, 616625.
The objective of this work was to study the catalytic gasification of a subbituminous coal from the Powder River Basin (PRB) using a CO2 and H2O mixture as the gasifying agent.
Semantic Scholar extracted view of "Gasification of a South Australian lowrank coal with carbon dioxide and steam: kinetics and reactivity studies" by D. Ye et al. ... Catalytic gasification of a Powder River Basin coal with CO2 and H2O mixtures. ... This work reports on a kinetic study on the gasification of Brazilian mineral coal with steam ...
In this experimental and modeling investigation, Wyodak coal, a subbituminous coal from the Powder River Basin, was the coal employed and corn stover was the biomass. Torrefied corn stover was ...
A kinetic characterization of the CO 2 gasification of chars from Chinese lowrank lignite coal is performed by isothermal thermogravimetry. The isothermal condition is 1,073 K, and the CO 2 concentration range is 1090%. Alkali and alkali earth catalysts were used to promote the gasification reactivity.
Most of the coal produced in the PRB supports electric power generation in the United States. Starting in the 1990s, many coalfired power plants switched to subbituminous coal from the PRB—which has relatively low sulfur content—to meet tightening Clean Air Act emission 2003, the Powder River Basin yielded more coal than the Appalachian coal basins in the eastern United States.
As the largest coal mining region and the main coal supply in the United States, Powder River Basin (PRB) coal has a tight connection with this country's power industry and requires special attention in coal gasification studies. Very little investigation of PRB gasification rates in the presence of both CO 2 and steam have been done. As a ...
Multiple sources of carbon can be used for CO 2 gasification. Coal from varying ranks has been used ... SubBituminous Powder River Basin coal: Pure Char: SCM: 700900: : 74: : TGA [137] Fe Pure Char ... (1X) + ∑ n k cn k nc and k cn are the rate constants for the noncatalytic and catalytic gasification, respectively. k cn ...
CO2 gasification of a subbituminous Wyodak coal from the Powder River Basin (PRB) was conducted in a fixedbed laboratory gasifier at atmospheric pressure with FeCO3 as a catalyst precursor.
1. Introduction. Gasification technology offers one of the cleanest ways for different carbonaceous feedstocks. Since the 21st century, the C1 chemical industry based on syngas has developed rapidly under the promotion of largescale coal gasification technology, especially in a country rich in coal resources. 1 With the development of gasification technology, the feedstock of gasifiers ...
Competition and Inhibition Effects during Coal Char Gasification in the Mixture of H2O and CO2. Rui Zhang, Q. H. Wang, Zhongyang Luo, M. Fang, K. Cen. Chemistry. 2013. The mechanisms of char gasification in the mixture of H2O and CO2 are not clear, and some problems are yet to be solved. The LangmuirHinshelwood (LH) model of char ...
DOI: / Corpus ID: ; Catalytic CO 2 gasification of a Powder River Basin coal article{Zhang2015CatalyticC2, title={Catalytic CO 2 gasification of a Powder River Basin coal}, author={Fan Zhang and Deping Xu and Yonggang Wang and Yan Wang and Gao Ying and T. Popa and Maohong Fan}, journal={Fuel Processing Technology}, year={2015}, volume={130}, pages={107116} }
The objective of this work was to study the catalytic gasification of a subbituminous coal from the Powder River Basin (PRB) using a CO2 and H2O mixture as the gasifying agent. Sodium...
The objective of this work was to study the catalytic gasification of a subbituminous coal from the Powder River Basin (PRB) using a CO2 and H 2O mixture as the gasifying agent. Sodium and iron, in the form of inexpensive compounds, were chosen to catalyze the coal gasification.
Catalytic gasification in the coal conversion process is a promising way to develop ... Wang, Y., Argyle, M. D. Fan, M. CO 2 gasification of powder river basin coal catalyzed by a costeffective ...
Authors: Zhang, Fan; Xu, Deping; Wang, Yonggang; Wang, Yan; Gao, Ying; Popa, Tiberiu; Fan, Maohong Publication Date: Sun Feb 01 00:00:00 EST 2015 Sponsoring Org ...
A study on the effect of the CO2/steam mixtures and the addition of natural minerals on the reactivity of Adaro coal gasification. International ... Gasification of biomass with CO2 and H2O mixtures in a catalytic fluidised bed. ... Competition between H 2 O and CO 2 during the gasification of Powder River Basin coal. Fuel 2017, 187, 94102 ...
Gasification of biomass with CO 2 and H 2 O mixtures in a catalytic fluidised bed. Fuel 2017, 210, 605610. DOI: / Ying Wang, David A. Bell. Competition between H 2 O and CO 2 during the gasification of Powder River Basin coal. Fuel 2017, 187, 94102. DOI: /
![[PDF] Catalytic gasification of a Powder River Basin coal with CO2 and ...](/g3j1tlu/219.jpg)
The gasification experiments of coal chars with CO2 were carried out isothermally, with K, Ca, Ni, and Zn chloride catalysts, adopting a thermal gravimetric analyzer (TGA) from 800 to 1100 C. The. Expand 1 1 Excerpt CO2 gasification of Yangchangwan coal catalyzed by ironbased waste catalyst from indirect coalliquefaction plant
Catalytic gasification of a Wyodak lowsulfur subbituminous coal from the Powder River Basin of Wyoming was investigated using an inexpensive catalyst, Na2CO3, widely available in Wyoming.
The catalytic mechanism is generally described as the added metal element contacting with gasifying agent (H 2 O and/or CO 2 ) produces hydrogen and/or carbon monoxide and a layer of...
Electrochemical catalytic coal gasification experiments with Fuxin (FX) coal under a CO2 atmosphere were conducted to evaluate the effects of power and temperature on coal gasification and char structure evolution during electrochemical catalytic gasification (ECG). When the power was 400 W, with temperature increasing from 800 to 1000 °C, the CO content in the gas products increased by % ...
The objective of this research was to examine the mechanisms of FeCO 3, Na 2 CO 3, and FeCO 3Na 2 CO 3 based catalytic coal gasification of a lowsulfur subbituminous Wyodak coal from the Powder River Basin (PRB) of Wyoming. Xray diffraction (XRD), Möss spectroscopy, scanning electron microscopy (SEM), Fourier transform infrared spectroscopy (FTIR), gas chromatography (GCMS) and ...
CO2 gasification of Powder River Basin coal catalyzed by a costeffective and environmentally friendly iron catalyst journal, May 2015. Zhang, Fan; Xu, Deping; Wang, Yonggang; ... (GPE) concept for producing synthetic natural gas and hydrogen from coal involves the catalytic gasification of coal and carbon. GPE's technology "refines" coal ...
The YN coal samples were manually ground and sieved to particle sizes mm. The pyrolysis of coal samples and char gasification was carried out in a fixed bed reactor. The experimental setup is shown in Fig. 1. The quartz tube used in this work has an inner diameter of 5 cm and length of 22 cm, the
A study was carried out in both inert and CO 2 atmosphere to investigate the interaction mechanism of K 2 CO 3 with graphite and coal char during the catalytic gasification of coal char. The formation of K 2 CO 3 catalytic precursors was identified by using series of different techniques. The results obtained in an inert atmosphere show that the interaction between K 2 CO 3 and carbon readily ...
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